简介

先进碳材料与能源化学课题组(GRE@C)


高鑫,北京大学助理教授,研究员,博士生导师,海外高层次人才计划获得者。2018年博士毕业于北京大学化学与分子工程学院(导师:张锦 院士),2019-2023年在美国斯坦福大学材料系从事博士后研究(合作导师:Prof. Yi Cui),2023年加入北京大学材料科学与工程学院(张锦院士团队)。在Nature Nanotechnology, Science Advances, Advanced Materials, Chemical Society Reviews, Journal of the American Chemical Society, Proceedings of the National Academy of Sciences 等杂志发表论文30余篇,总引用4000余次。曾获北京大学优秀博士论文,博士研究生国家奖学金、北京大学校长奖学金等奖励,出版学术专著《石墨双炔薄膜的合成方法与应用探索》。

本课题组主要围绕碳基纳米材料的结构控制制备与能源化学开展创新性研究,主要研究方向包括(1)碳基纤维材料的控制制备与结构功能一体化;(2)新型碳材料石墨炔的控制制备与应用探索;(3)高能量密度二次电池的设计与开发。


代表性工作

1. X. Gao#, Z. Yu#, J. Wang, X. Zheng, Y. Ye, H. Gong, X. Xiao, Y. Yang, Y. Chen, S. E. Bone, L. C. Greenburg, P. Zhang, H. Su, J. Affeld, Z. Bao*, Y. Cui*, Electrolytes with moderate lithium polysulfide solubility for high-performance long-calendar-life lithium–sulfur batteries. Proc. Natl. Acad. Sci. 2023, 120, e2301260120.

2. X. Zheng#, X. Gao#, R. A. Vilá, Y. Jiang, J. Wang, R. Xu, R. Zhang, X. Xiao, P. Zhang, L. C. Greenburg, Y. Yang, H. L. Xin, X. Zheng, Y. Cui*. Hydrogen-substituted graphdiyne-assisted ultrafast sparking synthesis of metastable nanomaterials. Nat. Nanotechnol. 2023, 18, 153-159.

3. X. Gao, X. Zheng, Y. Tsao, P. Zhang, X. Xiao, Y. Ye, J. Li, Y. Yang, R. Xu, Z. Bao, Y. Cui*. All-solid-state lithium–sulfur batteries enhanced by redox mediators. J. Am. Chem. Soc. 2021, 143, 18188-18195.

4. X. Gao, X. Zheng, J. Wang, Z. Zhang, X. Xiao, J. Wan, Y. Ye, L. Chou, H. K. Lee, J. Wang, R. A. Vilá, Y. Yang, P. Zhang, L. Wang, Y. Cui*. Incorporating the nanoscale encapsulation concept from liquid electrolytes into solid-state lithium–sulfur batteries. Nano Lett. 2020, 20, 5496-5503.

5. X. Gao, H. Liu, D. Wang, J. Zhang*. Graphdiyne: synthesis, properties, and applications. Chem. Soc. Rev. 2019, 48, 908-936.

6. X. Gao#, Y. Zhu#, Y. Ding, J. Zhou, S. Zhang, C. Yin, F. Ding, S. Zhang, X. Yi, J. Wang, L. Tong*, Y. Han*, Z. Liu*, J. Zhang*. Ultrathin graphdiyne film on graphene through solution-phase van der Waals epitaxy. Sci. Adv. 2018, 4, eaat6378.

7. X. Gao#, J. Li#, R. Du, J. Zhou, M. Huang, R. Liu, J. Li, Z. Xie, L. Wu*, Z. Liu*, J. Zhang*. Direct synthesis of graphdiyne nanowalls on arbitrary substrates and its application for photoelectrochemical water splitting cell. Adv. Mater. 2017, 1605308.

8. X. Gao#, H. Ren#, J. Zhou, R. Du, C. Yin, R. Liu, H. Peng, L. Tong*, Z. Liu*, J. Zhang*. Synthesis of hierarchical graphdiyne-based architecture for efficient solar steam generation. Chem. Mater. 2017, 29, 5777-5781.

9. J. Li#, X. Gao#, X. Jiang, X. Li, Z. Liu, J. Zhang*, C. Tung, and L. Wu*. Graphdiyne: A Promising Catalyst–Support To Stabilize Cobalt Nanoparticles for Oxygen Evolution. ACS Catal. 2017, 28, 5209-5213.

10. X. Gao, J. Zhou , R. Du , Z. Xie , S. Deng , R. Liu, Z. Liu*, J. Zhang*. Robust Superhydrophobic Foam: A Graphdiyne-BasedHierarchical Architecture for Oil/Water Separation. Adv. Mater. 2016, 28, 168-173.

11. J. Li#, X. Gao#, B. Liu, Q. Feng, X. Li, M. Huang, Z. Liu, J. Zhang*, C. Tung, Li. Wu*. Graphdiyne: A metal-free material as hole transfer layer to fabricate quantum dot-sensitized photocathodes for hydrogen production. J. Am. Chem. Soc. 2016, 138, 3954-3957.

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